A basic introduction to frequency modulation in Pd and a video tutorial for building an fm patch . A demonstration of the Yamaha DX7. An extensive discussion of the properties of frequency modulation from Barry Truax (with links to examples from his compositions using this technique). And a technical explanation of FM with illustrations of the sidebands and more from another master of the technique - Bill Schottstaedt.
Several illustrations of configuration for fm-synthesis sounds (bell-like, brass-like, etc.). A general tutorial about fm-synth with reference to various software implementations.
This method was pioneered by John Chowning. Here he is explaining how he discovered this technique:
His piece Stria applies the Golden Ratio to constructing its fm-synthesised tones.
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